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CO2 capture from atmospheric air via consecutive CaO-carbonation and CaCO3-calcination cycles in a fluidized-bed solar reactor

Author(s): Nikulshina V, Gebald C, Steinfeld A

Published: February, 2009

Publisher: Chemical Engineering Journal

DOI: 10.1016/j.cej.2008.06.005

Tags: Air Capture

URL: http://www.sciencedirect.com/science/article/pii/S1385894708003550

Abstract: A thermochemical cyclic process and associated reactor is presented for the continuous removal of CO2 from ambient air via consecutive CaO-carbonation and CaCO3-calcination steps using concentrated solar energy as the source of high-temperature process heat. A fluidized-bed solar reactor is applied to accomplish the carbonation at 365–400 °C and the calcination at 800–875 °C, with reacting particles directly exposed to high-flux solar irradiation. Water vapor was introduced during the carbonation step to enhance its kinetics. Five consecutive cycles were performed, yielding complete removal of CO2 from a continuous airflow containing 500 ppm of CO2 within a residence time of 1.3 s during each carbonation step, and subsequent complete release of CO2 and regeneration of the CaO reacting particles during the calcination step. The reactor design, set-up, and experimentation using a high-flux solar simulator are described.


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